Ultraslow dynamics and stress relaxation in the aging of a soft glassy system

Abstract

We use linear rheology and multispeckle dynamic light scattering (MDLS) to investigate the aging of a gel composed of multilamellar vesicles. Light scattering data indicate rearrangement of the gel through an unusual ultraslow ballistic motion. A dramatic slowdown of the dynamics with sample age $t_{w}$ is observed for both rheology and MDLS, the characteristic relaxation time scaling as $t_{w}^μ$. We find the same aging exponent $μ=0.78$ for both techniques, suggesting that they probe similar physical processes, that is the relaxation of applied or internal stresses for rheology or MDLS, respectively. A simple phenomenological model is developed to account for the observed dynamics.

8 pages, 4 figures, Submitted to PRL