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Direct Observation of the Quantum Energy Gap in S = 1/2 Tetragonal Cuprate Antiferromagnets

arXiv:cond-mat/0008009 · doi:10.1209/epl/i2001-00276-4

Abstract

Using an electron spin resonance spectrometer covering a wide range of frequency and magnetic field, we have measured the low energy excitations of the S=1/2 tetragonal antiferromagnets, Sr_{2}CuO_{2}Cl_{2} and Sr_{2}Cu_{3}O_{4}Cl_{2}. Our observation of in-plane energy gaps of order 0.1 meV at zero external magnetic field are consistent with a spin wave calculation, which includes several kinds of quantum fluctuations that remove frustration. Results agree with other experiments and with exchange anisotropy parameters determined from a five band Hubbard model.

4 pages, 3 figures