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Femtosecond two-photon-excited backward lasing of atomic hydrogen in flame

arXiv:1711.06875 · doi:10.1364/OL.43.001183

Abstract

We report on an observation of bi-directional 656 nm lasing action of atomic hydrogen in premixed CH4/air flame induced by resonant femtosecond 205 nm two-photon excitation. In particular, the backward-propagating lasing pulse is systematically characterized in the spectral, spatial and temporal domains for the sake of single-ended diagnostic. Its picosecond-scale duration enables spatially resolved concentration measurements of hydrogen atoms in millimeter range, which is successfully demonstrated using two narrow welding flames.

13 pages, 5 figures, submitted to Optica