Temperature Dependence of Nonlinear Susceptibilities in an Infinite Range Interaction Model

Abstract

We present a model to probe metamagnetic properties in systems with an arbitrary number of interacting spins. Thermodynamic properties such as the magnetization per particle $m(B,T,N)$, linear susceptibility $χ_1(T)$, nonlinear susceptibilities $χ_3(T)$ and $χ_5(T)$, specific heat $C(B,T,N)$, and pressure $P(B,T,N)$ were calculated. The model produces a different magnetic response for $N$ particles when comparing to $N - 1$ particles for small $N \sim 1$. For an even number of particles, the susceptibilities show maxima in their temperature dependence. An odd number produces an additional free spin response that dominates at low temperatures. This free spin response for odd $N$ also produces a step in the magnetization per particle at $B = 0$. The magnetization shows $N/2$ steps at $γB_c/J = n$ with integer $n$ for even $N$ and $(N-1)/2$ additional steps at half-integer $n$ starting at 3/2 for odd $N$. Small clusters respond with metamagnetism in an otherwise isotropic spin space, while the large clusters show no metamagnetism.