Neutron scattering study of a quasi-2D spin-1/2 dimer system Piperazinium Hexachlorodicuprate under hydrostatic pressure

Abstract

We report inelastic neutron scattering study of a quasi-two-dimensional S=1/2 dimer system Piperazinium Hexachlorodicuprate under hydrostatic pressure. The spin gap Δ becomes softened with the increase of the hydrostatic pressure up to P= 9.0 kbar. The observed threefold degenerate triplet excitation at P= 6.0 kbar is consistent with the theoretical prediction and the bandwidth of the dispersion relation is unaffected within the experimental uncertainty. At P= 9.0 kbar the spin gap is reduced to 0.55 meV from 1.0 meV at ambient pressure.

4 pages, 5 figures