Detection of the Meissner Effect with a Diamond Magnetometer

Abstract

We examine the possibility of probing superconductivity effects in metal nanoclusters via diamond magnetometry. Metal nanoclusters have been proposed as constitutive elements of high T$_c$ superconducting nanostructured materials. Magnetometry based on the detection of spin-selective fluorescence of nitrogen-vacancy (NV) centers in diamond is capable of nanoscale spatial resolution and could be used as a tool for investigating the properties of single or multiple clusters interacting among each other or with a surface. We have carried out sensitivity estimates and experiments to understand how these magnetometers could be used in such a situation. We studied the behavior of the sensor as a function of temperature and detected the flux exclusion effect in a superconductor by monitoring the [111]-orientation fine structure spectrum in high-NV density diamond. Our results show that phase transitions can be ascertained in a bulk superconductor with this technique while the principal zero field splitting parameter ($D$) demonstrates a temperature dependence that may require compensation schemes.