Quantum Imaging of Topologically Unpaired Spin-Polarized Dirac Fermions

Abstract

The motion of a relativistic particle is linked to its spin by the Dirac equation. Remarkably, electrons in two-dimensional materials can mimic such Dirac particles but must always appear in pairs of opposite spin chirality. Using topological ideas of chiral boundary electrons wrapping a three-dimensional crystal with tuned spin-orbit coupling, we show that elusive unpaired Dirac fermions exist on the surface of a topological insulator parent matrix, pure antimony. Using scanning tunneling microscopy and angle-resolved photoemission spectroscopy we image coherent quantum interference between these particles, map their helical spin texture, and ultimately observe a transition to a single Dirac fermion distinguished by backscattering suppression via Berry phase interference. The robust dynamics of these unique spin-polarized carriers envisage future applications in spintronics and topological quantum computation.

Updated from original (copy of earlier journal submission) to include references and context to latest published and posted experiments involving STM and ARPES