The nature of the magnetic and structural phase transitions in BaFe$_{2}$As$_{2}$

Abstract

We present the results of an investigation of both the magnetic and structural phase transitions in a high quality single crystalline sample of the undoped, iron pnictide compound BaFe$_2$As$_2$. Both phase transitions are characterized via neutron diffraction measurements which reveal simultaneous, continuous magnetic and structural orderings with no evidence of hysteresis, consistent with a single second order phase transition. The onset of long-range antiferromagnetic order can be described by a simple power law dependence $ϕ(T)^2\propto(1-\frac{T}{T_N})^{2β}$ with $β=0.103\pm0.018$; a value near the $β=0.125$ expected for a two-dimensional Ising system. Biquadratic coupling between the structural and magnetic order parameters is also inferred along with evidence of three-dimensional critical scattering in this system.

New figure and discussion added. Length: 11 pages, 7 figures