Large nonlinear absorption and refraction coefficients of carbon nanotubes estimated from femtosecond Z-scan measurements
arXiv:0710.2721 · doi:10.1063/1.2825409
Abstract
Nonlinear transmission of 80 and 140 femtosecond pulsed light with $0.79 μm$ wavelength through single walled carbon nanotubes suspended in water containing sodium dodecyl sulphate is studied. Pulse-width independent saturation absorption and negative cubic nonlinearity are observed, respectively, in open and closed aperture Z-scan experiments. The theoretical expressions derived to analyze the z-dependent transmission in the saturable limit require two photon absorption coefficient $β_0\sim$ $1.4 cm/MW$ and a nonlinear index $γ\sim -5.5 \times10^{-11} cm^2/W$ to fit the data.
10 pages, 2 figures. Accepted and to appear in Applied Physics Letters