Effects of Rattling Phonons on the Quasiparticle Excitation and Dynamics in the Superconducting $β$-Pyrochlore KOs$_2$O$_6$

Abstract

Microwave penetration depth $λ$ and surface resistance at 27 GHz are measured in high quality crystals of KOs$_2$O$_6$. Firm evidence for fully-gapped superconductivity is provided from $λ(T)$. Below the second transition at $T_{\rm p}\sim 8$ K, the superfluid density shows a step-like change with a suppression of effective critical temperature $T_{\rm c}$. Concurrently, the extracted quasiparticle scattering time shows a steep enhancement, indicating a strong coupling between the anomalous rattling motion of K ions and quasiparticles. The results imply that the rattling phonons help to enhance superconductivity, and that K sites freeze to an ordered state with long quasiparticle mean free path below $T_{\rm p}$.

5 pages, 5 figures, to be published in Phys. Rev. Lett